Final Program Banyuls-sur-mer Sept. 25-28, 2001 General Information

Combustion / Marangoni Convection

Dynamics / Diffusion & Growth Invited Lectures
Microgravity Application Program (MAP) / Biotechnology /. Spin-Offs / ESA Programmes Biology / Neurobiology / Dev. Biology / Technology / Sounding Rocket Program Human Physiology / Cell Biology
Plant Biology Posters ELGRA Medals

COMBUSTION / MARANGONI CONVECTION

FUNDAMENTAL ANALYSIS ON FLAME PROPAGATION BEHAVIOR AT LEAN LIMIT MIXTURES USING MICROGRAVITY TECHNIQUE

S. Okajima and A.Okajima
Faculty of Engineering, Hosei University, J-184 8584 Tokyo, Japan

From the viewpoint of low air pollution and energy saving on the combustion equipments such as international combustion engines, it is very important to elucidate the combustion behaviour of lean limit mixtures near the flammability limit.
Thus, experiments have been carried out to examine the characteristics of flame propagation close to the lean limit mixtures in a closed bomb by using the microgravity technique. The flame characteristics are studied by realizing the spherical flame propagation in a closed bomb under microgravity. Of course, microgravity techniques make it possible to obtain the fundamental combustion properties even for very lean mixtures because the symmetrical flame behaviour, by eliminating the buoyancy effect, can be achieved by a microgravity technique. Microgravity environment is achieved in a free fall facility of 490 m drop shaft in JAMIC (Japan Microgravity Center) located in Kamisunagawa, Hokkaido, Japan. The gravity level of the combustion chamber inside the falling capsule is 0.00001g. The falling assembly contains a cylindrical combustion bomb, an igniter, a schlieren photographic system and a camera unit. The cylindrical combustion bomb has 116 mm in diameter and 120 mm in length, which is equipped with a concave mirror and a Pyrex glass window on the opposite walls along the optical axis.
Experiments have been performed at room temperature and an initial pressure of 0.1 MPa. The fuels used are methane and propane of 99.9% purity. The main conclusions of the study are as follows: (1) microgravity techniques make it possible to determine very slow burning velocities with high accuracy, (2) the minimum value of burning velocity obtained for methane-air mixtures at 293 K and 0.1 MPa has been evaluated as 3.58 cm/s in the vicinity of 0.48 of equivalence ratio, (3) the cellular flame can be observed at very lean methane-air mixtures, and(4) the irregular flame propagation occurs when the Lewis number is less than the unity for propane-air mixtures only.
Key Words: Microgravity, Lean limit mixtures, Burning velocity, Lewis number, Irregular flame behaviour.

EFFECTS OF WIND AND OXYGEN CONCENTRATION ON A LAMINAR DIFFUSION FLAME ESTABLISHED OVER A HORIZONTAL FLAT PLATE IN MICRO-GRAVITY ENVIRONMENT

H. Y. Wang, P. Corderio, P. Joulain and J. Torero
Laboratoire de Combustion et de Détonique , C.N.R.S. UPR 9028 -E.N.S.M.A., Université de Poitiers, BP 109 - Site du Futuroscope, 86960, Futuroscope Cedex, France

Fire propagation over a condensed fuel in a micro-gravity environment is of particular interest in a human-occupied spacecraft. The condensed fuel vaporises due to heat transfer from the flame to the surface through radiation and convection. The fuel exothermically reacts with the oxidiser and provides the necessary heat to sustain further pyrolysis.
An experimental and numerical investigation of a laminar diffusion flame established over a horizontal flat plate in micro-gravity environment is described. Fuel is injected through the burner and the oxidiser (air) is provided by a forced flow parallel to the surface. The experiments were conducted in a range of oxygen concentration from 23 to 30% at two different wind velocities of 2.6 and 4 cm/s in a 5 s drop tower. The flame experiments make use of a pilot wire to ignite the sample in normal-gravity environment. It is observed that after the imposition of the micro-gravity, a plume region is maintained momentarily due to the dominant inertia. The transition time is about 2.5 s for reducing the overall air flow velocity to that of the forced boundary layer flow.
Direct Numerical Simulation (DNS) is used to provide a detailed description of the transition process of the flame in micro-gravity environment. The main advantage lies in the identification of the delay time for reducing an oscillated pool-like flame to a boundary layer flame type in micro-gravity condition. High enough spatial and temporal resolution with an efficient flow solving technique is needed for describing the flame structure during the transition period. The computational grid is fine enough to resolve the diffusion of fuel and oxygen. The starting point of the analysis is the set of three-dimensional, partial differential equations that governs the phenomena of interest here. The combustion process is described by a global one-step, finite-rate reaction given by the Arrhenius expression. This set consists, in general, of the following equations: the continuity equation, the three momentum equations that govern the conservation of momentum per unit mass in each of the three space dimensions, the equations for conservation of chemical species and of soot formation, and the radiative transfer equation. The finite-difference method is used to discretize the appropriate three-dimensional conservation equations. The parameters varied are the oxygen concentration and oxidiser flow velocity. The model results reflect the qualitative features of the experiments.


COMBUSTION STUDY ON SOLID WASTE FUELS IN HIGH TEMPERATURE ENVIRONMENT USING MICROGRAVITY TECHNIQUE

A. Okajima and S. Okajima
Faculty of Engineering, Hosei University, J-184 8584 Tokyo, Japan

From the viewpoint of effective use in the combustion furnaces of the solid waste fuels produced from an industrial field, it is very important to examine the combustion behaviour of solid waste fuels in high temperature environments. Thus, the authors have made an attempt at two kinds of combustion experiments of solid waste fuels under microgravity achieved in a freely falling capsule. One is for elucidating the combustion characteristics in high temperature environments and other one is for studying the influence of oxygen concentration on flame development in room temperature and in a very small air flow. The combustion behaviour of solid waste fuels is observed by taking direct photographs with an
8-mm video camera installed on the falling capsule.
The test facility employed in the study contains an electrical furnace, an 8-mm video camera, an air cylinder, a temperature control equipment of electrical furnace, a delay device and a back light system. The electrical furnace is a rectangular shape of 110 x 110 mm having 150 mm in length. The shape of the solid waste fuel is a sphere ranging from 2 to 3 mm in diameter.
Experiments have been conducted in high temperature environment ranging from 800K to 1100K, in ambient temperature and 0.1 MPa in ambient pressure. The microgravity environment of 10 second is realized by free fall facilities of 490 m drop shaft in JAMIC (Japan Microgravity Center). The main results show that,
(1) there are three categories for the combustion behaviour of solid waste fuels in a high temperature environment, that is ignition, luminous diffusion flame and smoldering process, (2) above 900K the ignition occurs with a very strong luminous flame and the complete combustion process is achieved throughout the smoldering process; on the contrary, below 850K it almost takes the smoldering process (surface combustion), (3) the ignition delay decreases monotonically with increasing ambient temperature, (4) even for very small air velocity it is very effective to enhance the combustion rate, and (5) the decrease of oxygen concentration at room temperature markedly makes a change for the worse in the combustion process.
Key Words: Solid waste fuels, Ignition delay, Luminous diffusion flame, Smoldering.

FIRST MEASUREMENT OF GAS TEMPERATURES BASED ON LIF OF FORMALDEHYDE

1
A. Burkert, 2J. König, 1W. Triebel
1 Institut für Physikalische Hochtechnologie e.V., Winzerlaer Straße 10,
D-07745 Jena, Germany
2 ZARM, University of Bremen, Am Fallturm, D-28359 Bremen, Germany

The reduction of air pollution e.g. from internal combustion engines and gas turbines is an important task. Drop tower facilities equipped with optical diagnostic systems are an approved tool to derive an advanced knowledge and understanding of the kinetics in combustion processes as cool flame phase and two-stage ignition [1, 2]. The two-dimensional detection of different species as e.g. formaldehyde (HCHO) [3] during the combustion process and the derivation of concentration and temperature fields are necessary to verify and develop reduced reaction kinetics of technical fuels. HCHO is a well-known tracer for knocking in internal combustion engines and is mainly present in the cool flame stage of ignition [4]. Nevertheless, the derivation of concentration fields of formaldehyde is difficult, mainly attributed to the quenching of fluorescence and to the lacking of non-intrusive techniques for temperature measurements under cool flame conditions.
In this paper we present a technique for temperature measurement under cool flame conditions based on laser induced fluorescence (LIF) of formaldehyde. The spectroscopic LIF and PLIF investigations of HCHO were performed with a set-up consisting of a double-tube XeF excimer laser, an optical multi-channel analyser, two intensified CCD cameras (ICCD) and hot calibration cells [1, 3]. A detailed LIF investigation of formaldehyde under different temperatures, pressures and concentrations revealed a temperature dependence of the ratio of the spectral regions from 390...400 nm to 390...418 nm. A system dependent calibration function can be obtained by recording of LIF spectra of formaldehyde under controlled temperature conditions in a high-pressure gas cell and determining the LIF-ratio from 390...400 nm to 390...418 nm.
First temperature measurements based on LIF of formaldehyde were performed in a pre-heated measurement cell including a small porous sphere filled with liquid n-heptane. For this purpose a laser light sheet was formed to excite formaldehyde in the cool flame phase of ignition. LIF images were recorded with two ICCD cameras, which were equipped with specially designed filters.
In addition, we discuss modifications of the laser diagnostic system at the drop tower of Bremen, which are necessary to apply this new method of measurement of temperature fields and to investigate ignition processes in more detail under microgravity conditions.
- König J., Eigenbrod Chr., Rath H.J., Grebner D., Hein J., Triebel W., "Formaldehyde-PLIF detection of cool-flame reactions during two stage ignition of alkane droplets", 5th Intl. Microgravity Combustion Workshop, Cleveland 18-20th May 1999
- König, J., Eigenbrod, Chr., Rath, H.J., Grebner, D. Hein, J., Triebel, W., "Formaldehyde-PLIF Detection of Cool-Flame Reactions During Two Stage Ignition of Alkane Droplets", 5th Intl. Microgravity Combustion Workshop, NASA/CP-1999-208917, 189, 1999
- Burkert A., Grebner D., Müller D., Triebel W., König J., "Single shot imaging of formaldehyde in hydrocarbon flames by XeF excimer laser induced fluorescence", Twenty-Eighth Symposium (International) on Combustion, The Combustion Institute, Pittsburgh, PA, 2000, pp. 135-141
- Bäuerle B., Warnatz J., Behrend F., Twenty-Sixth Symposium (International) on Combustion, The Combustion Institute, Pittsburgh, PA, 1996, pp. 2619-2626


SIMULATION OF GEOPHYSICAL FLUID FLOWS UNDER MICROGRAVITY

C. Egbers, P. Chossat and R. Hollerbach
University of Technology, LAS, Karl-Liebknecht-Strasse 102, D-03046 Cottbus, Germany

The objective of this research programme is to study thermally-driven rotating fluids, in order to investigate the stability, pattern formation, and transition to turbulence of incompressible fluids trapped between concentric, co-axially rotating spheres.
The physical mechanisms addressed in this proposal are important for a large number of astrophysical and geophysical problems having spherical geometry flows shaped by rotation and convection: for example, to explain the mantle convection of the earth, the differential rotation effect on the sun, the zonal atmospheric jets on the giant planets, or the flow in a planet’s interior (like the earth). Understanding and controlling fluid flow in a spherical geometry under the influence of rotation will also be useful in a variety of engineering applications, such as improving spherical gyroscopes and bearings, and centrifugal pumps. Furthermore, study of effects related to the electro-hydrodynamic force, which serves to simulate the central gravity field in the space experiments, will find applications in high-performance heat exchangers, and in the study of electro-viscous phenomena. It will also help to understand the motion of liquids in several ground-based industrial applications where injected ions are a source of charge, e.g. in electrostatic precipitators and ion-drag pumps.
The experimental set-up is performed to investigate the problems of thermal convection in the fluid shell between two concentric half-spheres with and without rotation, and also with differentially rotating spheres (around the same axis). A central symmetric force field similar to the gravity field acting on planets can be produced by applying a high voltage potential between the inner and outer sphere, using the effect of dielectrophoretic force field.

THERMOCAPILLARY FLOW STRUCTURES UNDER MICROGRAVITY IN A LONG FLOATING ZONE (NEAR THE RAYLEIGH LIMIT)

D. Schwabe
Physical Institute of the University of Giessen, 35392 Giessen, Germany

The length L and the "ideal" shape of floating zones is limited to some mm under normal gravity (1-g) due to hydrostatic pressure. Therefore, the hydrothermal waves of oscillatory thermocapillary flow can only travel in azimuthal direction, which allows for wavelengths l j up to » 2p R, with R the zone radius. Axial components l z are suppressed or frustrated because L << 2p R under 1-g. The theory for infinitely long zones by Xu and Davis, Phys. Fluids 27 (1984) 1102, predicts much smaller critical Marangoni numbers for the onset of oscillations Mac = -¶ s /¶ T × h -1 × c -1 × R2 × ¶ T/¶ z and different oscillation periods from what is found under normal gravity in short floating zones. This is most likely due to the end effects in small – L floating zones which do not allow the most dangerous states with axial components of the hydrothermal waves.
Under microgravity (m -g) non-deformed floating zones of a length up to the Rayleigh limit Lmax = 2p R are possible, giving an aspect ratio Amax = L/R = 2p » 6.28. In such a zone the axial and the azimuthal space for the development of a hydrothermal wave is the same and one can expect to observe and measure l z besides l j , different frequencies and a smaller Mac of the most dangerous mode.
We have realized an A = 5 floating zone from silicone oil (2 cSt, Pr = 29) under microgravity during the 14 min. ballistic phase of the sounding rocket MAXUS-4 (29.04.2001). We installed 4 different supercritical Marangoni numbers and came to fully relaxed flow states because of the small zone dimensions (R = 3.0 mm, L = 15.0 mm). The flow was observed by tracer motion in a vertical and in a horizontal light sheet. The oscillation amplitude was measured with very fine thermocouples placed 0.7 mm below the free surface (wire Æ =
25 m m); -5 thermocouples placed at different axial positions but the same azimuth, 4 placed in different azimuthal positions but the same z.
We report on the measured Mac, the frequencies at supercritical Ma, the mode number and the axial and the radial component of the hydrothermal wave in this unique object. The measurements are discussed in comparison to the predictions of theory and the hydrothermal wave is visualized with a video-clip.

DYNAMIC FREE-SURFACE DEFORMATIONS DUE TO HYDROTHERMAL WAVES IN THERMOCAPILLARY LIQUID BRIDGES

H. C. Kuhlmann and Ch. Nienhüser
ZARM - University of Bremen, Am Fallturm, D-28359 Bremen, Germany

The physical mechanism for the onset of oscillations in thermocapillary flows has long been discussed controversially. It is now well established that the transition to oscillatory flows in moderately high-Prandtl-number liquid bridges is caused by the hydrothermal-wave instability mechanism, if the mean surface tension is asymptotically large. According to another hypothesis, the dynamic deformability of the liquid-gas interface is required, for oscillatory flow to occur in high-Prandtl-number fluids. Some investigations are underway to measure the dynamic free-surface deformations and to relate these to the flow and temperature fluctuations. In this presentation dynamic surface deformations are considered to
leading order in an expansion for small capillary numbers, i.e. for small relative variation of the surface tension. It has been found that the dynamic surface deformations associated with the critical oscillatory flow decouple, at leading order, from the dynamic deformations of the axisymmetric basic flow. Therefore, the dynamic deformability is not responsible for the instability for small capillary numbers. Using a numerical analysis, we have predicted the shape of the deformations caused by the critical oscillatory mode and determined their amplitude relative to that of the associated surface-temperature fluctuations.
Acknowledgments:
This work has been supported by DLR and by NASDA. We are indebted to S. Yoda for his continued encouragement.